I think this would be a nice addition to have, but this would probably not go over well with the wider GNOME app development community, as a lot of them are very vocal against third-party theming by distributions (see: stopthemingmy.app) (and I sense this also extends to DE-level theming)
If we are gonna do it at all, I think we should make it opt-in, probably with some warning like “some applications might break from this, and if it does, please do not bother the app maintainer!”
I didn’t imply adding it to KDE/Plasma, gtk3-nocsd wasn’t added either, after all. However, I do plan to incorporate gtk3-nocsd into this and making it as seamless as possible and would be proud if it was added, but I do agree that the Gnome side wouldn’t be happy about it. So I just recommended it for people that want to try it and add it to their own installs